Table 2.
Summary of free energy values for CLC-ec1 dimerization in 2:1 POPE/POPG lipid bilayers
Monomer/dimer distributionsΔWTΔW
 kcal/mol kcal/mol 
PM: 400-nm EPL Walden (KD = 1 × 10100−11.4 ± 0.2 (0.84) −9.5 ± 0.2 (0.85) 
PD: 400-nm EPL Walden (KD = 1 × 10−100  
PM: 400-nm 2:1 POPE/POPG (KD = 1 × 10100−11.3 ± 0.2 (0.70) −8.4 ± 0.2 (0.45) 
PD: 400-nm 2:1 POPE/POPG (KD = 1 × 10−100  
PM: WW −10.7 ± 0.2 (0.75) −8.5 ± 0.2 (0.80) 
PD: WT + glutaraldehyde   
PM: WW −10.9 ± 0.1 (0.90) −8.8 ± 0.2 (0.83) 
PD: R230C/L249C   
Monomer/dimer distributionsΔWTΔW
 kcal/mol kcal/mol 
PM: 400-nm EPL Walden (KD = 1 × 10100−11.4 ± 0.2 (0.84) −9.5 ± 0.2 (0.85) 
PD: 400-nm EPL Walden (KD = 1 × 10−100  
PM: 400-nm 2:1 POPE/POPG (KD = 1 × 10100−11.3 ± 0.2 (0.70) −8.4 ± 0.2 (0.45) 
PD: 400-nm 2:1 POPE/POPG (KD = 1 × 10−100  
PM: WW −10.7 ± 0.2 (0.75) −8.5 ± 0.2 (0.80) 
PD: WT + glutaraldehyde   
PM: WW −10.9 ± 0.1 (0.90) −8.8 ± 0.2 (0.83) 
PD: R230C/L249C   

Free energies are calculated as ΔG° = −RT ln(Keq χ°), where χ° is the mole fraction standard state of 1 subunit/lipid, R is the gas constant 1.99 × 10−3 kcal mole−1 K−1, and T is 298 K (25°C), where Keq (lipids/subunit) is determined by fitting to the equilibrium dimerization isotherm. Data represent best-fit ± error of fit (R2). KD, dissociation constant (subunit/lipid) equal to 1/Keq; PM, nonreactive monomer distribution; PD, nonreactive dimer distribution.

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